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Disentangling structural and dynamical effects via multidimensional high harmonic spectroscopy

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Abstract

Extending the dimensionality of high harmonic generation (HHG) measurements has the potential to reconstruct structural features in molecules and resolve multielectron dynamics on attosecond time scales. We demonstrate that structural and dynamical effects in molecules can be unambiguously distinguished using multidimensional HHG techniques.

© 2014 Optical Society of America

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