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Ultrafast and Photodissociation Dynamics of 1,2-Butadiene Studied by Photoelectron Spectroscopy

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Abstract

Ultrafast and photodissociation dynamics of a cumulated dine molecule, 1,2-butadiene, were investigated by time-resolved photoelectron spectroscopy using a high harmonic. In contrast with 1,3-butadiene, coherent oscillation by stimulated Raman process was observed prior to photodissociation.

© 2014 Optical Society of America

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