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The Ultrafast Wolff Rearrangement in the Gas Phase

Andreas Steinbacher, Sebastian Roeding, Tobias Brixner, and Patrick Nuernberger

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Abstract

The sub-picosecond Wolff rearrangement of gas-phase 5-diazo Meldrum’s acid is disclosed with femtosecond ion spectroscopy. Distinct differences are found for 267 nm and 200 nm excitation, the latter leading to even two ultrafast rearrangement reactions.

© 2014 Optical Society of America

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