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Visible Two-Dimensional Spectroscopy with sub-7 fs Pulses Uncovers Ultrafast Electron-Phonon Coupling Dynamics

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Abstract

Electronic two-dimensional spectroscopy with sub-7 fs resolution with the aid of simulations and quantum chemistry reveals the time scale and underlying dynamics of electron-phonon coupling, internal vibrational redistribution, and double quantum resonances in solvated Zinc-Phthalocyanine.

© 2010 Optical Society of America

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