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Highly Exergonic Bimolecular Electron Transfer Beyond Marcus Theory, the Importance of Molecular Structure and Dynamics

Bernhard Lang, Katrin Adamczyk, Natalie Banerji, Diego Villamaina, Jens Dreyer, Erik T. J. Nibbering, and Eric Vauthey

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Abstract

The combination of visible and mid infrared transient absorption yields a direct insight into structural dynamics and determination of distinct reaction pathways in highly exergonic electron transfer, asking for refinement of existing theories.

© 2010 Optical Society of America

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