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Probing Ultrafast Dynamics of 5f Electrons in Crystalline UO2

Y. Q. An, A. J. Taylor, T. Durakiewicz, and G. Rodriguez

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Abstract

We find the lifetimes of photoexcited 5f electrons in crystalline UO2, ~1.2 ns for midgap states and ~2 µs for upper Hubbard band states at low temperatures, identify magnetic transitions, and observe picosecond intraband relaxation.

© 2010 Optical Society of America

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