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Probing electron transfer in polymer/fullerene blends using ultrahigh time resolution coherent vibrational spectroscopy

S. M. Falke, D. Brida, G. Cerullo, and C. Lienau

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Abstract

We report nonlinear optical spectra of polymer/fullerene-blends measured with unprecedented 10-fs-time resolution. Our results suggest that the photoinduced charge-generation in such blends proceeds via a hybrid electronic state delocalized over the polymer and fullerene moieties.

© 2010 Optical Society of America

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