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Separating Sub-Ensembles on Ultrafast Timescales: Multiple-Population Period Transient Spectroscopy (MUPPETS)

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Abstract

Multidimensional incoherent spectroscopy has analogs of echoes, stimulated echoes, hole-burning and correlation spectroscopy. These MUPPETS methods disentangle complex, nonexponential kinetics. A pathway formulation extends MUPPETS to many processes and systematically treats high-order transient gratings.

© 2010 Optical Society of America

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