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Ultrafast Conversions of Hydrogen-Bonded Structures in Liquid Water Observed via Femtosecond Soft X-ray Spectroscopy

N. Huse, H. Wen, H. Cho, T.-K. Kim, R.W. Schoenlein, and A.M. Lindenberg

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Abstract

X-ray spectroscopic studies relate distinct spectral features to water molecules in lose and tight H-bond environments. Femtosecond x-ray measurements show that vibrational excitation/relaxation increases weakly H-bonded water at the direct expense of tightly H-bonded water.

© 2010 Optical Society of America

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