Picosecond X-ray Absorption Spectroscopy of Photochemical Transient Species in Solution

Munira Khalil; Matthew A. Marcus; Amanda L. Smeigh; James K. McCusker; Henry H. W. Chong; Robert W. Schoenlein

doi:10.1364/UP.2006.WD5

15th International Conference on Ultrafast Phenomena
OSA Technical Digest Series (CD) (Optica Publishing Group, 2006),
paper WD5
•https://doi.org/10.1364/UP.2006.WD5

Picosecond X-ray Absorption Spectroscopy of Photochemical Transient Species in Solution

Munira Khalil, Matthew A. Marcus, Amanda L. Smeigh, James K. McCusker, Henry H. W. Chong, and Robert W. Schoenlein

International Conference on Ultrafast Phenomena 2006

Pacific Grove, California United States
31 July–4 August 2006
ISBN: 1-55752-810-1

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Chemistry and X-Rays (WD)

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M. Khalil, M. A. Marcus, A. L. Smeigh, J. K. McCusker, H. H. W. Chong, and R. W. Schoenlein, "Picosecond X-ray Absorption Spectroscopy of Photochemical Transient Species in Solution," in 15th International Conference on Ultrafast Phenomena, OSA Technical Digest Series (CD) (Optica Publishing Group, 2006), paper WD5.

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Abstract

A photoinduced Fe^Π spin crossover reaction in solution is studied with ultrafast x-ray absorption spectroscopy. The iron-nitrogen bond lengthens by 0.21±0.03 Å in the high-spin transient excited state relative to the ground state.

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