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Rotational wave packet dynamics correlated to ultrafast non-time-stationary linear and nonlinear optical susceptibilities

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Abstract

Rotational wave packet dynamics produced by a ultrafast alignment pulse are related to linear and nonlinear optical susceptibilities. Limitations of wave packet dynamic probing through optical susceptibilities are revealed. Correlations between nonlinear order and fractional revivals are discussed.

© 2006 Optical Society of America

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