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Decomposing the Excited State Dynamics of Carotenoids in Light Harvesting Complexes and Dissecting Pulse Structures from Optimal Control Experiments

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Abstract

Dispersed transient absorption and multi-pump spectroscopies were used to illustrate how the interplay between excited-state dynamics, saturation, and annihilation phenomena in the LH2 protein from Rhodopseudomonas acidophila generates structured pulses in optimal control experiments.

© 2006 Optical Society of America

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