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Real-time Investigation of Elementary Steps for Photo-induced Phase Transition in a Model Dimer

L. Lüer, C. Manzoni, G. Cerullo, G. Lanzani, and M. Meneghetti

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Abstract

Using femtosecond pump and probe spectroscopy and ab-initio calculations, we show that photoexcitation of dimers of tetramethyl-tetrathiafulvalene cations induces predominantly coherent phonons that lead to photoinduced phase transitions in linear chains of these materials.

© 2006 Optical Society of America

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