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Ultrafast Gigantic Photo-Response in (EDO-TTF)2PF6 Initiated by 10-fs Laser Pulses

Jiro Itatani, Matteo Rini, Andrea Cavalleri, Ken Onda, Tadahiko Ishikawa, Shin-ya Koshihara, Xiangfeng Shao, Hideki Yamochi, Gunzi Saito, and Robert W. Shoenlein

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Abstract

We photoexited a charge-ordered organic salt (EDO-TTF)2PF6 with sub-10-fs optical pulses. The photo-induced metallic phase appeared within 50-fs after pumping, characterized by large changes in reflectivity (ΔR/R∼0.8) followed by strong coherent phonon modulation.

© 2006 Optical Society of America

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