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Conferences > UP > 2006 > MI > MI11

Manipulating Multidimensional Nonlinear Electronic Spectra of Excitons by Coherent Control with Polarization Pulse Shaping

Dmitri V. Voronine, Shaul Mukamel, and Darius Abramavicius

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Abstract

Femtosecond two-pulse photon echo signals of excitons from a chiral porphyrin dimer are simulated using the cumulant expansion method. Off-diagonal peaks are amplified and resolved, and diagonal peaks are suppressed by using coherent control with adaptive polarization pulse shaping combined with a genetic algorithm.

© 2006 Optical Society of America

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