Two-dimensional optical heterodyne spectroscopy of molecular complexes

Igor Stiopkin; Tobias Brixner; Graham R. Fleming

14th International Conference on Ultrafast Phenomena
Technical Digest (CD) (Optica Publishing Group, 2004),
paper TuB5

Two-dimensional optical heterodyne spectroscopy of molecular complexes

Igor Stiopkin, Tobias Brixner, and Graham R. Fleming

International Conference on Ultrafast Phenomena 2004

Niigata Japan
25–30 July 2004
ISBN: 3-54024-110-8

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Multidimensional Spectroscopy (TuB)

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I. Stiopkin, T. Brixner, and G. R. Fleming, "Two-dimensional optical heterodyne spectroscopy of molecular complexes," in 14th International Conference on Ultrafast Phenomena, Technical Digest (CD) (Optica Publishing Group, 2004), paper TuB5.

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Abstract

Optical heterodyne two-dimensional (2D) photon echoes from room-temperature BIC J-aggregates were recorded. Analysis of the time-dependent 2D spectrum reveals the frequency dependence of the exciton relaxation, and discriminates diagonal and off-diagonal exciton phonon coupling.

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