Abstract
Polarization-dependent transient infrared spectroscopy probes the restricted ultrafast orientational motion of CO inside the Xe4 cavity of myoglobin. The four-point correlation function 〈μ(0)μ(0)μ(T)μ(T+t)〉 does not factorize and only its full evaluation reproduces the observed anisotropies.
© 2004 Optical Society of America
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