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  • 14th International Conference on Ultrafast Phenomena
  • Technical Digest (CD) (Optica Publishing Group, 2004),
  • paper ThD19

Restricted rotational motion of CO in a protein internal cavity: observation of non-separating four-point correlation functions by IR pump-probe spectroscopy

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Abstract

Polarization-dependent transient infrared spectroscopy probes the restricted ultrafast orientational motion of CO inside the Xe4 cavity of myoglobin. The four-point correlation function 〈μ(0)μ(0)μ(T)μ(T+t)〉 does not factorize and only its full evaluation reproduces the observed anisotropies.

© 2004 Optical Society of America

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