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Optica Publishing Group
  • The Thirteenth International Conference on Ultrafast Phenomena
  • 2002 OSA Technical Digest Series (Optica Publishing Group, 2002),
  • paper ME20
  • https://doi.org/10.1364/UP.2002.ME20

Time-resolved photoelectron-photoion coincidence imaging of the photodissociation and ionization dynamics in CF3I

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Abstract

The real-time dynamics of the dissociative ionization of CF3I has been studied by femtosecond photoelectron-photoion coincidence imaging. With coincidence imaging, correlated three dimensional scattering data of the recoiling electrons and the parent ion, CF3+ and I+ photofragment are obtained. With the photoelectron spectra of CF3I+ and the correlated images of the fragments, the different multi-photon dissociation pathways producing I+ are unravelled. Furthermore, molecular frame angular correlations are extracted for the CF3+ and I+ photofragments. These molecular frame angular correlations provide details on the photodissociation and ionization dynamics.

© 2002 Optical Society of America

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