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Femtosecond Dynamics of Pyridine in the Condensed Phase: Valence Isomerization by Conical Intersections

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Abstract

In this work, we combined femtosecond transient absorption spectroscopy with ab initio electronic structure methods to study deactivation pathways of pyridine molecule in solutions. A conical intersection was found responsible for the ultrafast deactivation.

© 2000 Optical Society of America

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