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Early events in the photoexcitation of π-conjugated chains studied with sub-10-fs time resolution

G. Cerullo, M. Zavelani-Rossi, G. Lanzani, and S. De Silvestri

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Abstract

Using sub-10-fs pulses, pump-probe experiments were carried out on prototypical it-conjugated chains belonging to the class of carotenoids and semiconducting polymers. The internal-conversion rate and the subsequent excited state thermalization are directly measured.

© 2000 Optical Society of America

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