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Femtosecond multicolor pump-probe investigations of ultrafast electron transfer of (NH3)5RuIIINCRuII(CN)5 in aqueous solution

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Abstract

Ultrafast measurements on aqueous (NH3)5RuIIINCRuII(CN)5 reveal an ultrafast spectral component due to vibrationally unrelaxed stimulated emission, allowing for new insights on the interplay of solvent and solute degrees of freedom in an electron transfer reaction.

© 2000 Optical Society of America

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