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  • Conference on Lasers and Electro-Optics/Quantum Electronics and Laser Science Conference and Photonic Applications Systems Technologies
  • OSA Technical Digest (CD) (Optica Publishing Group, 2008),
  • paper JWD1

Single-Shot, Space- and Time-Resolved Measurement of Rotational Wavepacket Revivals in H2 and D2

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Abstract

Femtosecond laser induced alignment and periodic recurrences of room temperature hydrogen and deuterium molecules are measured in a single shot for the first time, using single-shot supercontinuum spectral interferometry (SSSI). The measurements are also performed in oxygen and some other common linear molecular gases. Employing time-dependent first order perturbation theory, an analytical model of rotational wavepacket revivals is derived, which shows good agreement with the experiment.

© 2008 Optical Society of America

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