Coherent transient spectroscopy of CO adsorbed on Cu(111)

J. C. Owrutsky; J. P. Culver; M. Li; Y. R. Kim; M. Sarisky; M. S. Yeganeh; A. G. Yodh; R. M. Hochstrasser

Quantum Electronics and Laser Science Conference
OSA Technical Digest (Optica Publishing Group, 1992),
paper QFC4

Coherent transient spectroscopy of CO adsorbed on Cu(111)

J. C. Owrutsky, J. P. Culver, M. Li, Y. R. Kim, M. Sarisky, M. S. Yeganeh, A. G. Yodh, and R. M. Hochstrasser

Quantum Electronics and Laser Science Conference 1992

Anaheim, California United States
10–15 May 1992
ISBN: 1-55752-540-5

From the session
Second Harmonic Studies of Surfaces (QFC)

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J. C. Owrutsky, J. P. Culver, M. Li, Y. R. Kim, M. Sarisky, M. S. Yeganeh, A. G. Yodh, and R. M. Hochstrasser, "Coherent transient spectroscopy of CO adsorbed on Cu(111)," in Quantum Electronics and Laser Science Conference, E. Ippen, S. Chu, J. Shah, and C. Weiman, eds., Vol. 13 of OSA Technical Digest (Optica Publishing Group, 1992), paper QFC4.

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Abstract

Coherent transient spectroscopy has provided important information on relaxation phenomena in gases, liquids, and solids. Recently, there has been intense interest in the vibrational dynamics of molecular adsorbates on simple surfaces.^1–4 In this contribution, we present free induction decay (HD) measurements of the vibrational dephasing of CO absorbed on Cu(111). To our knowledge this represents the first measurement of an HD signal from an adsorbate on a metal, and the fastest coherent transient ir measurement performed on surface adsorbates thus far.

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