Abstract
We have initiated the unimolecular reaction– by exciting the molecule to particular rotation- vibration levels in the ground electronic state. Excitation with a visible dye laser at 661 or 565 nm populates overtone levels of the NH stretch, vNH = 5 or 6, by direct overtone pumping. Nascent NH fragments are detected by laser-induced fluorescence (LIF).
© 1989 Optical Society of America
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