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Highly Nonlinear Femtosecond Processes in Liquid Phase: Water Cluster Raman Spectra and Microheterogeneity Induced Coherent Oscillations

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Abstract

Stokes region of water supercontinuum shows explicit water-cluster Raman features arising at high laser intensities. Near-infrared degenerate pump-probe of a cyanine dye shows coherent oscillations only in binary liquid mixtures at sub-40 femtosecond resolution.

© 2014 Optical Society of America

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