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Probing Exciton Couplings and Correlations in Semiconductors with Optical Two-Dimensional Fourier Transform Spectroscopy

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Abstract

We study many-body interactions between excitons in semiconductors by applying a new and powerful technique, optical two-dimensional Fourier transform spectroscopy. A single two-dimensional spectrum can identify couplings between resonances, separate quantum mechanical pathways, and distinguish among microscopic many-body interactions.

© 2007 Optical Society of America

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