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Conferences > LS > 2015 > LTu5G > LTu5G.3

Probing Buffer-Gas Cooled Molecules with Direct Frequency Comb Spectroscopy in the Mid-Infrared

B. Spaun, P. B. Changala, B. J. Bjork, O. H. Heckl, J. Ye, D. Patterson, and J. M. Doyle

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Abstract

We demonstrate cavity-enhanced direct frequency comb spectroscopy on buffer-gas cooled molecules. By coupling a mid-infrared frequency comb to a high-finesse cavity surrounding a 4 K buffer-gas chamber, we obtain rotationally resolved absorption spectra of multiple vibrational bands of nitromethane.

© 2015 Optical Society of America

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