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Comparison of Electronic and Vibrational Coherence Measured by Two-Dimensional Electronic Spectroscopy

Daniel B. Turner and Gregory D. Scholes

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Abstract

We measured broadband two-dimensional electronic spectra of a laser dye, a quantum dot, and an algal photosynthetic protein. We determined the origin of the cross peak oscillations by investigating the nonrephasing contribution in each system.

© 2011 Optical Society of America

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