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The Role of Nuclear Modes in Coupled Electronic Systems: Quantum Coating, Vibronic Modulation, or Quantum-Dissipative Energy Flow?

N. Christensson, O. Bixner, F. Milota, J. Hauer, and H. F. Kauffmann

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Abstract

The modulation of electronic dynamics by nuclear modes in a phthalocyanine dimer has been investigated by 2D-ES. Quantum-dissipative relaxation between the two excited states on 20 fs timescale is mediated by a 700 cm−1mode.

© 2011 Optical Society of America

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