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Two Dimensional Femtosecond Stimulated Raman Spectroscopy: A New Technique to Probe Vibrational Coupling

David W. McCamant, Kristina C. Wilson, Randy D. Melenbacher, and Brendon Lyons

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Abstract

Two-dimensional femtosecond stimulated Raman spectroscopy (2D-FSRS) can potentially quantify vibrational coupling. However, our results indicate that all signals measured thus far are attributable to a 3rd-order cascade and not the intended 5th-order mechanism.

© 2010 Optical Society of America

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