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Observation of Intra-molecular Vibrational Dynamics using High-Harmonic Generation as a Probe

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Abstract

Intra-molecular vibrational dynamics in SF6 are observed, using electrons rescattered during the process of high-order harmonic generation. All of the Raman- active modes of SF6 are observed, as well as vibrational relaxation.

© 2006 Optical Society of America

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