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Theory of Single-Pulse Femtosecond Coherent Anti-Stokes Raman Scattering Using a Chirped Probe Beam

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Abstract

The theory of single-pulse, chirped-probe, femtosecond (fs) coherent anti-Stokes Raman scattering (CARS) for gas-phase temperature and species measurements is developed. The time-dependent density matrix equations are solved numerically for the fs CARS process.

© 2008 Optical Society of America

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