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  • 2013 Conference on Lasers and Electro-Optics - International Quantum Electronics Conference
  • (Optica Publishing Group, 2013),
  • paper CFIE_1_1

The influence of nuclear motion on the electron dynamics in an efficient sub-cycle control of the molecule K2

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Abstract

With precise control of the temporal phase of femtosecond laser pulses direct manipulation of valence electron motion is possible. The control scheme relies on the selective population of dressed states first demonstrated for atoms [1]. In a combined experimental and theoretical approach, we show that the control scheme can be transferred to molecules. For the example of the potassium dimer specific target states can be addressed through the control of the electron dynamics. The key element is the oscillating dipole created by the superposition of the X1Σg+ ground state and the A1Σu+ first excited state. We highlight the effect of the nuclear motion on the control scheme and in particular on the oscillating dipole.

© 2013 IEEE

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