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Conferences > IQEC > 1990 > QWI > QWI2
  • International Quantum Electronics Conference
  • OSA Technical Digest (Optica Publishing Group, 1990),
  • paper QWI2

Picosecond free radical chemistry in clusters: (CH3I)n à state excitation

J. A. SYAGE and J. STEADMAN

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Abstract

The combination of picosecond resonance-enhanced multiphoton ionization (REMPI)1,2 and direct ion photodissociation3,4 holds great promise for studying complex reaction mechanisms in size-specific neutral and ionic dusters. We applied these techniques to the study of free radical chemistry initiated by picosecond à state excitation in (CH3I)n clusters.1 Picosecond mass-selective measurements of rapid duster photochemistry provide a new domain for studying the molecular basis of solvation on reactive systems.

© 1990 Optical Society of America

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