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Conferences > IQEC > 1990 > QTHC > QTHC3
  • International Quantum Electronics Conference
  • OSA Technical Digest (Optica Publishing Group, 1990),
  • paper QTHC3

Picosecond acid-base chemistry in dusters: phenol-(NH3)n

J. STEADMAN and J. A. SYAGE

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Abstract

The use of molecular clusters is proving to be an excellent medium for studying stepwise solvation.1-4 However, the existing body of work comprises steady state experiments.1-2 which are sensitive only to the equilibria of reactant and product. We report direct picosecond measurements of the rate constants for acid dissociation ka and geminate recombination k–a as a function of solvent cluster size for the seeded cluster system phenol-(NH3)n (henceforth ROH • Mn).3

© 1990 Optical Society of America

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