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Optica Publishing Group
  • International Quantum Electronics Conference
  • OSA Technical Digest (Optica Publishing Group, 1984),
  • paper MHH5

Interferometrie Enhancement of Surface-Generated Second-Harmonic Radiation

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Abstract

Second-harmonic (SH) generation from dye monolayer coverages adsorbed on fused-silica substrates has been demonstrated recently.12 It has also been shown that this effect can be greatly enhanced if the harmonic light is at resonance with the S1-S2 band-to-bandtransition of the dye molecules. With a spectral enhancement of up to a factor 100, this technique of surface spectroscopy may be used to characterize the adsorbed monolayer with respect to the nature of the adsorbate and its coverage density.

© 1984 Optical Society of America

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