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Probing the transition from hydrophilic to hydrophobic solvation with atomic scale resolution

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Abstract

We use ultrafast x-ray absorption spectroscopy to determine the solvent structure change upon laser abstraction of the electron from I-. The transition from hydrophilic to hydrophobic occurs over 4 ps during which a transient I-OH2 species is formed.

© 2012 Optical Society of America

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