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Spectroscopy of the Lowest Two-Photon Transition for Molecules in Solution by Automated DFWM

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Abstract

We use degenerate four-wave mixing with wavelength-tunable picosecond pulses to study the second hyperpolarizability of molecules in solution. The full dispersion of both real and imaginary parts of the polarizability can be obtained using a semi-automated method.

© 2015 Optical Society of America

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