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Role of Saturation of Rotational Raman Transition on Femtosecond Vibrational CARS

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Abstract

Saturation of femtosecond vibrational Raman coherence and coherent anti-Stokes Raman scattering (CARS) signal in air show drastically different characteristic compared to nanosecond regime. Rotational Raman saturation is shown to dictate the behavior of vibrational Raman.

© 2013 Optical Society of America

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