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Conferences > CLEO_QELS > 2017 > FTh3F > FTh3F.2

Strong Local-Field Enhancement of the Nonlinear Softmode Response in Aspirin

Giulia Folpini, Klaus Reimann, Michael Woerner, Thomas Elsaesser, Johannes Hoja, and Alexandre Tkatchenko

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Abstract

Softmode excitations in aspirin are studied with two-dimensional terahertz spectroscopy. The coupling of CH3 rotational modes and collective excitations of π electrons results in a nonperturbative nonlinear response induced by moderate THz fields.

© 2017 Optical Society of America

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