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Optical Pump - Multi-THz Probe Spectroscopy of a Single Crystal Organic Hybrid Lead Halide Perovskite

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Abstract

We analyzed ultrafast photocarrier generation in single crystal CH3NH3PbI3 perovskite through time-resolved terahertz spectroscopy. We find a Drude-Lorentz type conductivity spectra with a carrier mobility of 35 cm2/Vs and a Lorentzian component at 45 meV possibly due to intra-excitonic transitions.

© 2015 Optical Society of America

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