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Conferences > CLEO_Europe > 2015 > CG_6 > CG_6_5
  • 2015 European Conference on Lasers and Electro-Optics - European Quantum Electronics Conference
  • (Optica Publishing Group, 2015),
  • paper CG_6_5

Laser pulse duration can control the breakage of multiple chemical bonds

Xinhua Xie, Erik Lötstedt, Stefan Roither, Sonia Erattupuzha, Seyedreza Larimian, Daniil Kartashov, Markus Schöffler, Katsumi Midorikawa, Andrius Baltuška, Kaoru Yamanouchi, and Markus Kitzler

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Abstract

Using ethylene (C2H4) as an example, we experimentally demonstrate control of complex fragmentation reactions that involve the breakage of more than one chemical bond using ultrashort intense laser pulses with pulse durations from 4.5 fs to 25 fs. We show that the dynamics of removing three electrons by strong-field ionization determines the ratio of fragmentation of the molecular trication into two respectively three moieties.

© 2015 IEEE

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