Abstract
Time-resolved four-wave mixing (FWM) has been widely implemented in the study of the third-order nonlinear optical susceptibility in semiconductors.1 As a third-order process, FWM has been shown to be sensitive to multiphoton excitations, which are difficult to observe with linear optical spectroscopy.2 Two-photon (TP) absorption and more generally, multiphoton absorption have been studied extensively in semiconductors.3 When a semiconductor is excited below its single-photon band gap, in particular, near midgap, TP nonlinearities become important.4 To the best of our knowledge, however, the contribution of the TP third-order nonlinearity has not been previously studied in semiconductors. It has been studied, however, in molecular solutions and polymers.5
© 1995 Optical Society of America
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