Rotary echo measurement of dipole transition matrix elements

Tao-Heng Sun; M.-K. Kim; E. L. Hahn

doi:10.1364/CLEO.1985.WN5

Conference on Lasers and Electro-Optics
OSA Technical Digest (Optica Publishing Group, 1985),
paper WN5
•https://doi.org/10.1364/CLEO.1985.WN5

Rotary echo measurement of dipole transition matrix elements

Tao-Heng Sun, M.-K. Kim, and E. L. Hahn

Conference on Lasers and Electro-Optics 1985

Baltimore, Maryland United States
21–24 May 1985
ISBN:

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Spectroscopy (WN)

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T. Sun, M. -. Kim, and E. L. Hahn, "Rotary echo measurement of dipole transition matrix elements," in Conference on Lasers and Electro-Optics, A. Gara, C. Giuliano, D. Auston, and R. Jacobs, eds., OSA Technical Digest (Optica Publishing Group, 1985), paper WN5.

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Abstract

The rotary echo in the IR region using the Stark switching technique¹ is applied to the measurement of an effective transition dipole matrix element of a ¹³CH₃F gas vibration–rotational transition. The experiment is performed by irradiating ¹³CH₃F gas with a cw CO₂ laser in the TEM₀₀ mode and switching the IR transitions of the molecule with dc Stark electric field pulses. The infrared ¹³CH₃F vibration-rotational transition involved is

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