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Conferences > CLEO > 1983 > TUD > TUD2

Stimulated Raman studies of low-frequency pure-spin Raman transltions to 3Σg ground state oxygen

Adelbert Owyoung, Ronald A. Hill, and Peter Esherick

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Abstract

The spin degeneracy of the ground 3Σg state of molecular oxygen is split due to spin-spin and spin-rotational interactions. These spin splittings result in spectral splittings in both the rotational and vibrational Raman bands of the molecule.1 Pure- spin transitions between these levels have also been observed directly by both spontaneous Raman2 and microwave spectroscopies.3 However, until now, only microwave techniques have been able to re- solve the spin transitions arising from individual rotational levels.

© 1983 Optical Society of America

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