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Efficient and Broadband Picosecond Stimulated Raman Scattering in KTiOPO4

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Abstract

Picosecond SRS with single-pass efficiency exceeding 50% and 34 THz bandwidth was observed in KTiOPO4. At peak intensities above 10 GW/cm2 the SRS character changes from narrowband to broadband showing substantial “softening” of polariton modes.

© 2006 Optical Society of America

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